All-coupling polaron optical response: Analytic approaches beyond the adiabatic approximation
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KLIMIN, Serghei, TEMPERE, Jacques, DEVREESE, Josef T.. All-coupling polaron optical response: Analytic approaches beyond the adiabatic approximation. In: Physical Review B, 2016, vol. 94, pp. 1-13. ISSN 2469-9950. DOI: https://doi.org/10.1103/PhysRevB.94.125206
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Physical Review B
Volumul 94 / 2016 / ISSN 2469-9950 /ISSNe 2469-9969

All-coupling polaron optical response: Analytic approaches beyond the adiabatic approximation

DOI:https://doi.org/10.1103/PhysRevB.94.125206

Pag. 1-13

Klimin Serghei12, Tempere Jacques13, Devreese Josef T.14
 
1 University of Antwerp,
2 Moldova State University,
3 Howard University,
4 Eindhoven University of Technology
 
 
Disponibil în IBN: 25 noiembrie 2022


Rezumat

In the present work, the problem of an all-coupling analytic description for the optical conductivity of the Fröhlich polaron is treated, with the goal being to bridge the gap in the validity range that exists between two complementary methods: on the one hand, the memory-function formalism and, on the other hand, the strong-coupling expansion based on the Franck-Condon picture for the polaron response. At intermediate coupling, both methods were found to fail as they do not reproduce diagrammatic quantum Monte Carlo results. To resolve this, we modify the memory-function formalism with respect to the Feynman-Hellwarth-Iddings-Platzman approach in order to take into account a nonquadratic interaction in a model system for the polaron. The strong-coupling expansion is extended beyond the adiabatic approximation by including in the treatment nonadiabatic transitions between excited polaron states. The polaron optical conductivity that we obtain at T=0 by combining the two extended methods agrees well, both qualitatively and quantitatively, with the diagrammatic quantum Monte Carlo results in the whole available range of the electron-phonon coupling strength.

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