Low-field magnetic properties of La1-xCaxMnO3 (0 ≤ x ≤ 0.4)
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Electromagnetism. Câmp electromagnetic. Electrodinamică (60)
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LAIHO, Reino, LISUNOV, Konstantin, LÄHDERANTA, Erkki, PETRENKO, Peter A., STAMOV, Vladimir, ZAKHVALINSKII, Vasilii. Low-field magnetic properties of La1-xCaxMnO3 (0 ≤ x ≤ 0.4). In: Journal of Magnetism and Magnetic Materials, 2000, vol. 213, pp. 271-277. ISSN 0304-8853. DOI: https://doi.org/10.1016/S0304-8853(00)00023-8
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Journal of Magnetism and Magnetic Materials
Volumul 213 / 2000 / ISSN 0304-8853

Low-field magnetic properties of La1-xCaxMnO3 (0 ≤ x ≤ 0.4)

DOI:https://doi.org/10.1016/S0304-8853(00)00023-8
CZU: 537.8

Pag. 271-277

Laiho Reino1, Lisunov Konstantin2, Lähderanta Erkki1, Petrenko Peter A.2, Stamov Vladimir2, Zakhvalinskii Vasilii2
 
1 Wihuri Physical Laboratory, University of Turku,
2 Institute of Applied Physics, Academy of Sciences of Moldova
 
 
Disponibil în IBN: 16 februarie 2024


Rezumat

Magnetic properties of cubic La1-xCaxMnO3 (0 ≤ x ≤ 0.4) are investigated between T = 5 and 310 K in the external field of 2 G. The dependence of the ferromagnetic transition temperature on x is analyzed with the model of spin polarons associated with electronic localization and electron-electron interaction. The bandwidth of the localized electrons is found to be W = 1.90 ± 0.05 eV. In the samples with x < 0.2 and the Mn4+ concentration c < 0.26, a transition to a canted antiferromagnetic spin state is observed. The dependence of the transition temperature, T1, on c can be well described by a model including the Mn3+-Mn3+ superexchange and the Mn3+-Mn4+ double-exchange interactions. In the samples with x ≤ 0.2 and c ≤ 0.22 the value of the critical exponent, γ = 1.21 ± 0.05, is obtained for the temperature dependence of the zero-field-cooled susceptibility function χ-1 (T) approx. (T - TC)γ, for T > TC.

Cuvinte-cheie
Engineering controlled terms Electrons, Lanthanum alloys, Magnetic fields, magnetic susceptibility, magnetization, Manganese alloys, Superconducting transition temperature Engineering uncontrolled terms Antiferromagnetic spin state, Electron electron interaction, Ferromagnetic transition temperature, Low field properties, Magnetic compounds, Spin polarons Engineering main heading Antiferromagnetic materials