Large ordered moment with strong easy-plane anisotropy and vortex-domain pattern in the kagome ferromagnet Fe3Sn
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PRODAN, Lilian, DONALD, M. Evans, GRIFFIN, Sinead M., OSTLIN, Andreas, ALTTHALER, Markus, LYSNE, Erik Nikolai, FILIPPOVA, Irina, SHOVA, Sergiu, CHIONCEL, L., TSURKAN, Vladimir, KEZSMARKI, Istvan. Large ordered moment with strong easy-plane anisotropy and vortex-domain pattern in the kagome ferromagnet Fe3Sn. In: Applied Physics Letters, 2023, vol. 123, p. 0. ISSN 0003-6951. DOI: https://doi.org/10.1063/5.0155295
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Applied Physics Letters
Volumul 123 / 2023 / ISSN 0003-6951

Large ordered moment with strong easy-plane anisotropy and vortex-domain pattern in the kagome ferromagnet Fe3Sn

DOI:https://doi.org/10.1063/5.0155295

Pag. 0-0

Prodan Lilian1, Donald M. Evans1, Griffin Sinead M.2, Ostlin Andreas1, Altthaler Markus1, Lysne Erik Nikolai3, Filippova Irina4, Shova Sergiu5, Chioncel L.1, Tsurkan Vladimir14, Kezsmarki Istvan1
 
1 Institut für Physik, Universität Augsburg,
2 Lawrence Berkeley National Laboratory,
3 Norwegian University of Science and Technology, Trondheim,
4 Institute of Applied Physics, MSU,
5 “Petru Poni” Institute of Macromolecular Chemistry
 
 
Disponibil în IBN: 15 august 2023


Rezumat

We report the magnetic anisotropy of kagome bilayer ferromagnet Fe3Sn probed by the bulk magnetometry and magnetic force microscopy (MFM) on high-quality single crystals. The dependence of magnetization on the orientation of the external magnetic field reveals strong easy-plane magnetocrystalline anisotropy and anisotropy of the saturation magnetization. The leading magnetocrystalline anisotropy constant shows a monotonous increase from K 1 ≈ − 1.0 × 10 6 J / m 3 at 300 K to − 1.3 × 10 6 J / m 3 at 2 K. Our ab initio electronic structure calculations yield the value of total magnetic moment of 7.1 μ B / f . u . and a magnetocrystalline anisotropy energy density of −0.57 meV / f . u . ( − 1.62 × 10 6 J / m 3 ) both being in reasonable agreement with the experimental values. The MFM imaging reveals micrometer-scale magnetic vortices with weakly pinned cores that vanish at the saturation field of ∼3 T applied perpendicular to the kagome plane. The observed vortex-domain structure is well reproduced by the micromagnetic simulations, using the experimentally determined value of the anisotropy and exchange stiffness. 

Cuvinte-cheie
Binary alloys, electronic structure, Ferromagnetic materials, ferromagnetism, Magnetic anisotropy, Magnetic fields, Magnetic moments, Magnetocrystalline anisotropy, saturation magnetization, single crystals, Superconducting materials, Tin alloys, Vortex flow