Spin excitations in frustrated A -site spinels investigated with inelastic neutron scattering
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KRIMMEL, Alexander, MUTKA, Hannu, KOZA, Michael Marek, TSURKAN, Vladimir, LOIDL, Alois. Spin excitations in frustrated A -site spinels investigated with inelastic neutron scattering. In: Physical Review B - Condensed Matter and Materials Physics, 2009, vol. 79, p. 0. ISSN 1098-0121. DOI: https://doi.org/10.1103/PhysRevB.79.134406
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Physical Review B - Condensed Matter and Materials Physics
Volumul 79 / 2009 / ISSN 1098-0121 /ISSNe 1550-235X

Spin excitations in frustrated A -site spinels investigated with inelastic neutron scattering

DOI:https://doi.org/10.1103/PhysRevB.79.134406

Pag. 0-0

Krimmel Alexander1, Mutka Hannu2, Koza Michael Marek2, Tsurkan Vladimir13, Loidl Alois1
 
1 Center for Electronic Correlations and Magnetism, University of Augsburg,
2 Institut Laue-Langevin, Grenoble,
3 Institute of Applied Physics, Academy of Sciences of Moldova
 
 
Disponibil în IBN: 27 iunie 2023


Rezumat

The magnetic ions of the A -site spinels M Al2 O4 (M=Mn,Fe,Co) form a diamond lattice which, by means of competing interactions, are subject to strong frustration effects. In this paper we present the outcome of inelastic neutron-scattering experiments to investigate the corresponding magnetic excitations. MnAl2 O4 exhibits the strongest magnetic exchange and reveals long-range magnetic order below TN =40 K with a well-defined spin-wave dispersion. In contrast, CoAl2 O4 and FeAl2 O4 do not show long-range order but the magnetic scattering corresponds to a liquidlike structure factor. Inelastic neutron scattering in CoAl2 O4 shows a dispersionlike structure indicating collective magnetic excitations, despite the absence of long-range magnetic order. This type of behavior corresponds to a cooperative paramagnet. The opening of a spin gap in FeAl2 O4 is observed at low temperatures. These three A -site spinels are located on the border of long-range magnetic order with distinct emergent behavior. The corresponding role of orbital degrees of freedom is discussed. 

Cuvinte-cheie
magnetism, Curie Temperature, Antiferromagnet