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SM ISO690:2012 SCHILBERTH, Felix L., UNGLERT, Nico, PRODAN, Lilian, MEGGLE, F., EBAD-ALLAH, Jihaan, KUNTSCHER, Christine A., TSIRLIN, Alexander A., TSURKAN, Vladimir, DEISENHOFER, Joachim, CHIONCEL, L., KEZSMARKI, Istvan, BORDACS, Sandor. Magneto-optical detection of topological contributions to the anomalous Hall effect in a kagome ferromagnet. In: Physical Review B, 2022, vol. 106, pp. 1-10. ISSN 2469-9950. DOI: https://doi.org/10.1103/PhysRevB.106.144404 |
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Physical Review B | ||||||
Volumul 106 / 2022 / ISSN 2469-9950 /ISSNe 2469-9969 | ||||||
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DOI:https://doi.org/10.1103/PhysRevB.106.144404 | ||||||
Pag. 1-10 | ||||||
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A single ferromagnetic kagome layer is predicted to realize a Chern insulator with quantized Hall conductance, which upon stacking can become a Weyl semimetal with a large anomalous Hall effect (AHE) and magneto-optical activity. Indeed, in the kagome bilayer material Fe3Sn2, a large AHE was detected. In order to directly probe the responsible band structure features, we measure the optical Hall conductivity spectra in addition to the diagonal optical conductivity over a broad frequency range. Since the former is the energy selective measure of the intrinsic contributions to the AHE, we identify their common origin with the help of momentum- and band-decomposed optical conductivity spectra obtained from first principles calculations. We find that low-energy transitions, tracing "helical volumes"in momentum space reminiscent of the formerly predicted helical nodal lines, substantially contribute to the AHE, which is further increased by contributions from multiple higher-energy interband transitions. Our study also reveals that in this kagome magnet, local Coulomb interactions lead to remarkable band reconstructions near the Fermi level. |
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Cuvinte-cheie Binary alloys, Calculations, Ferromagnetic materials, ferromagnetism, Hall effect, Iron alloys, Tin alloys |
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