Spin-lattice instability in the chromium sulfur spinel Fe 0.5Cu0.5Cr2S4
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KALVIUS, Georg Michael, HARTMANN, Olaf N., KRIMMEL, Alexander, WAGNER, Friedrich Ernst, WAPPLING, Roger W., TSURKAN, Vladimir, KRUG VON NIDDA, Hans Albrecht, LOIDL, Alois. Spin-lattice instability in the chromium sulfur spinel Fe 0.5Cu0.5Cr2S4. In: Journal of Physics Condensed Matter, 2008, vol. 20, pp. 1-7. ISSN 0953-8984. DOI: https://doi.org/10.1088/0953-8984/20/25/252204
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Journal of Physics Condensed Matter
Volumul 20 / 2008 / ISSN 0953-8984 /ISSNe 1361-648X

Spin-lattice instability in the chromium sulfur spinel Fe 0.5Cu0.5Cr2S4

DOI:https://doi.org/10.1088/0953-8984/20/25/252204

Pag. 1-7

Kalvius Georg Michael1, Hartmann Olaf N.2, Krimmel Alexander3, Wagner Friedrich Ernst1, Wappling Roger W.2, Tsurkan Vladimir34, Krug Von Nidda Hans Albrecht3, Loidl Alois3
 
1 Technical University Munich,
2 Uppsala University,
3 Center for Electronic Correlations and Magnetism, University of Augsburg,
4 Institute of Applied Physics, Academy of Sciences of Moldova
 
 
Disponibil în IBN: 6 martie 2024


Rezumat

Zero field μSR spectroscopy was applied to a polycrystalline sample of the ferrimagnetic sulfur spinel Fe0.5Cu0.5Cr 2S4 between 5 and 315 K. The temperature dependence of the interstitial magnetic field Bμ as well as the transverse and longitudinal relaxation rates were deduced. At around 100 K, the temperature dependence of the interstitial field exhibits a strong deviation from the expected Brillouin-like behavior together with a maximum of the transverse relaxation rate. These features are characteristic for a spin reorientation transition. This instability of the ferrimagnetic spin-lattice has not been reported previously. 57Fe Mössbauer data from the same sample show no irregularity in the temperature dependence of the Fe hyperfine field which could indicate that the spin reorientation involves primarily the Cr sublattice. Above and below the spin reorientation regime, disorder in the spin-lattice is sizable, but not excessive. At low temperatures, the spins are essentially static, spin dynamics sets in above the reorientation range. The μSR data are also complemented by new susceptibility and magnetization data taken on similar material.

Cuvinte-cheie
Engineering controlled terms Magnetic field effects, Polycrystalline materials, Relaxation processes, Sulfur Engineering uncontrolled terms Relaxation rates, Spin-lattice instability Engineering main heading Chromium