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![]() ZAHARKO, Oksana, CERVELLINO, Antonio, TSURKAN, Vladimir, CHRISTENSEN, Niels Bech, LOIDL, Alois. Evolution of magnetic states in frustrated diamond lattice antiferromagnetic Co ( Al1-x Cox ) 2 O4 spinels. In: Physical Review B - Condensed Matter and Materials Physics, 2010, vol. 81, p. 0. ISSN 1098-0121. DOI: https://doi.org/10.1103/PhysRevB.81.064416 |
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Physical Review B - Condensed Matter and Materials Physics | ||||||
Volumul 81 / 2010 / ISSN 1098-0121 /ISSNe 1550-235X | ||||||
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DOI:https://doi.org/10.1103/PhysRevB.81.064416 | ||||||
Pag. 0-0 | ||||||
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Using neutron powder diffraction and Monte Carlo simulations we show that a spin-liquid regime emerges at all compositions in the diamond-lattice antiferromagnets Co (Al1-x Cox) 2 O4. This spin-liquid regime induced by frustration due to the second-neighbor exchange coupling J2 is gradually superseded by antiferromagnetic collinear long-range order (k=0) at low temperatures. Upon substitution of Al3+ by Co3+ in the octahedral B site the temperature range occupied by the spin-liquid regime narrows and TN increases. To explain the experimental observations we considered magnetic anisotropy D or third-neighbor exchange coupling J3 as degeneracy-breaking perturbations. We conclude that Co (Al1-x Cox) 2 O4 is below the theoretical critical point J2 / J1 =1/8, and that magnetic anisotropy assists in selecting a collinear long-range ordered ground state, which becomes more stable with increasing x due to a higher efficiency of O-Co3+ -O as an interaction path compared to O-Al3+ -O. |
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Cuvinte-cheie magnetism, Curie Temperature, Antiferromagnet |
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