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![]() LAIHO, Reino, LÄHDERANTA, Erkki, SALMINEN, J., LISUNOV, Konstantin, ZAKHVALINSKII, Vasilii. Spin dynamics and magnetic phase diagram of La1-xCaxMnO3(0 < ∼ x < ∼ 0.15). In: Physical Review B - Condensed Matter and Materials Physics, 2001, vol. 63, p. 0. ISSN 1098-0121. DOI: https://doi.org/10.1103/PhysRevB.63.094405 |
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Physical Review B - Condensed Matter and Materials Physics | ||||||
Volumul 63 / 2001 / ISSN 1098-0121 /ISSNe 1550-235X | ||||||
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DOI:https://doi.org/10.1103/PhysRevB.63.094405 | ||||||
Pag. 0-0 | ||||||
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Spin dynamics of ceramic La1-xCaxMnO3 with x = 0, 0.05, and 0.15 and the relative Mn4+ concentration c = 0.18-0.22 is investigated by measurements of the ac susceptibility and the relaxation of the thermoremanent magnetization (TRM). The χac(T) function exhibits a transition from the paramagnetic to a mixed spin-glass and ferromagnetic phase. Below that is found a steep decrease and onset of the frequency dependence of χac(T), providing evidence for existence of a reentrant spin glass (RSG) phase. The dependence of the spin-glass freezing temperature, Tf, on f satisfies the conventional critical slowing-down law, τ/τ0=(Tf/TG-1)-zv with τ = 1/f, zv = 12 ± 2, τ0→ 10-12s and the glass temperature, TG, decreasing from 93 to 70.5 K when x is increased from 0 to 0.15. The relaxation rate S(t) of TRM has a clear maximum near a wait time tw→(2-4) × 103s and the function S(T) shows a sharp maximum near TG. The plots of S(T) exhibit a substantial decrease at T >TG while for T <TG they collapse into a single curve, as typical for mixed (TG < T < TC) and RSG phases, respectively. The observed spin dynamics agrees completely with the magnetic phase diagram (paramagnetic, mixed, and RSG phases with decreasing T) predicted recently for a system containing lattice disorder and competing superexchange and double exchange interactions. |
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