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SM ISO690:2012 LÄHDERANTA, Erkki, HAJDEU-CHICAROS, Elena, KRAVTSOV, Victor, SHAKHOV, Mikhail, STAMOV, Vladimir, BODNAR, Ivan V., ARUSHANOV, Ernest, LISUNOV, Konstantin. Electronic properties of Cu2(Zn, Cd)SnS4 determined by the high-field magnetotransport. In: New Journal of Physics, 2022, nr. 9(24), pp. 1-15. ISSN 1367-2630. DOI: https://doi.org/10.1088/1367-2630/ac8b9f |
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New Journal of Physics | ||||||
Numărul 9(24) / 2022 / ISSN 1367-2630 | ||||||
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DOI:https://doi.org/10.1088/1367-2630/ac8b9f | ||||||
Pag. 1-15 | ||||||
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Resistivity, ρ(T), and magnetoresistance (MR) are investigated in the Cu2Zn1−x Cdx SnS4 single crystals for compositions x ≡ Cd/(Zn + Cd) = 0.15-0.24, in the temperature range of T ∼ 50-300 K in pulsed magnetic fields of B up to 20 T. The Mott variable-range hopping (VRH) conductivity is established within wide temperature intervals lying inside ΔT M ∼ 60-190 K for different x. The deviations from the VRH conduction, observable above and below ΔT M, are connected to the nearest-neighbor hopping regime and to the activation on the mobility threshold of the acceptor band (AB) with width W ≈ 16-46 meV. The joint analysis of ρ(T) and positive MR permitted determination of other important electronic parameters. These include the localization radius, α ≈ 19-30 Å, the density of the localized states, g(μ) ≈ (1.6-21) × 1017 meV−1 cm−3 at the Fermi level μ, and the acceptor concentration, N A ∼ (6-8) × 1019 cm−3, for various x and in conditions of different vicinity of the investigated samples to the metal-insulator transition. In addition, details of the AB structure, including positions of μ and of the mobility threshold, E c, are found depending on the alloy composition. |
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