Variable-range hopping conductivity of La1-xSr xMn1-yFeyO3
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ZAKHVALINSKII, Vasilii, LAIHO, Reino, LASHKUL, Alexander V., LISUNOV, Konstantin, LÄHDERANTA, Erkki, NEKRASOVA, Yulia, PETRENKO, Peter A., STAMOV, Vladimir. Variable-range hopping conductivity of La1-xSr xMn1-yFeyO3. In: Journal of Physics Condensed Matter, 2011, vol. 23, pp. 1-9. ISSN 0953-8984. DOI: https://doi.org/10.1088/0953-8984/23/1/015802
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Journal of Physics Condensed Matter
Volumul 23 / 2011 / ISSN 0953-8984 /ISSNe 1361-648X

Variable-range hopping conductivity of La1-xSr xMn1-yFeyO3

DOI:https://doi.org/10.1088/0953-8984/23/1/015802

Pag. 1-9

Zakhvalinskii Vasilii12, Laiho Reino3, Lashkul Alexander V.1, Lisunov Konstantin41, Lähderanta Erkki1, Nekrasova Yulia2, Petrenko Peter A.4, Stamov Vladimir43
 
1 Lappeenranta University of Technology,
2 Belgorod State University,
3 Wihuri Physical Laboratory, University of Turku,
4 Institute of Applied Physics, Academy of Sciences of Moldova
 
 
Disponibil în IBN: 19 iunie 2024


Rezumat

The temperature dependence of the resistivity, ρ, of ceramic La 1-xSrxMn1-yFeyO3 (LSMFO) samples with x = 0.3 and y = 0.03, 0.15, 0.20 and 0.25 (or simply #03, #15, #20 and #25, respectively) is investigated between temperatures T ∼ 5 and 310 K in magnetic fields B up to 8 T. Metallic conductivity in #03 is changed eventually to activated in #25. In #15 and #20 the behavior of ρ(T) is more complicated, comprising of two extremes, divided by an interval of metallic behavior in #15, and two inflections of ρ(T) in #20 within similar intervals ΔT below ∼100 K. Mott variable-range hopping (VRH) conductivity is observed in #15 above the ferromagnetic Curie temperature, T C. In #20 the Mott VRH conductivity takes place in three different temperature intervals at T > TC, T close to TC and T < TC. In #25, the Mott VRH conductivity is observed in two different intervals, above and below TC, divided by an intermediate interval of the Shklovskii-Efros VRH conduction regime. Analysis of the VRH conductivity yielded the values of the localization radius, α, and the dependence of α and of the density of the localized states, g, near the Fermi level, on B. Above TC the localization radius in all samples at B = 0 has similar values, α ≈ 1.0-1.2 Å, which is enhanced to α ≈ 3.3 Å (#20) and 2.0 Å (#25) below TC. The sensitivity of α and g to B depend on y and T. The complicated behavior of the mechanisms of the hopping charge transfer, as well as of the microscopic parameters α and g, is attributable to different electronic and magnetic phases of LSMFO varying with temperature and Fe doping.

Cuvinte-cheie
Engineering controlled terms Charge transfer, ion exchange, Magnetic fields Engineering uncontrolled terms Conduction regime, Fe doping, Intermediate interval, Localized state, Magnetic phasis, Metallic behaviors, Metallic conductivity, Microscopic parameter, Mott variable-range hopping, Temperature dependence, Temperature intervals, Variable-range hopping, VRH conductivity Engineering main heading Manganese