Enhanced phonon lifetimes with optically controlled single molecules
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CEBAN, Victor, MACOVEI, Mihai. Enhanced phonon lifetimes with optically controlled single molecules. In: Journal of the Optical Society of America B: Optical Physics, 2024, vol. 41, pp. 216-221. ISSN 0740-3224. DOI: https://doi.org/10.1364/JOSAB.506974
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Journal of the Optical Society of America B: Optical Physics
Volumul 41 / 2024 / ISSN 0740-3224 /ISSNe 1520-8540

Enhanced phonon lifetimes with optically controlled single molecules

DOI:https://doi.org/10.1364/JOSAB.506974

Pag. 216-221

Ceban Victor, Macovei Mihai
 
Institute of Applied Physics, MSU
 
 
Disponibil în IBN: 29 ianuarie 2024


Rezumat

We have investigated the phonon dynamics of a single molecule embedded in a mechanical resonator made of an organic crystal. The whole system is placed in an optical resonator within the bad cavity limit. We have found that the optical control of the molecular population affects the phonon dynamics. Long-lived phonons are obtained when slowing down the decay dynamics of the molecule via modulation of the transition frequency. The discussed results are also valid for optomechanical setups based on other types of two-level emitters and mechanical resonators.

Cuvinte-cheie
Decay dynamics, Mechanical resonators, Molecular population, Optical control, Optically controlled, organic crystal, Phonon dynamics, Phonon lifetimes, Single Molecule, Transition frequencies