Ruddlesden-Popper interface in correlated manganite heterostructures induces magnetic decoupling and dead layer reduction
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BELENCHUK, Alexandr, SHAPOVAL, Oleg M., RODDATIS, Vladimir, BRUCHMANN-BAMBERG, V., SAMWER, Konrad H., MOSHNYAGA, Vasily T.. Ruddlesden-Popper interface in correlated manganite heterostructures induces magnetic decoupling and dead layer reduction. In: Applied Physics Letters, 2016, vol. 109, p. 0. ISSN 0003-6951. DOI: https://doi.org/10.1063/1.4971833
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Applied Physics Letters
Volumul 109 / 2016 / ISSN 0003-6951

Ruddlesden-Popper interface in correlated manganite heterostructures induces magnetic decoupling and dead layer reduction

DOI:https://doi.org/10.1063/1.4971833

Pag. 0-0

Belenchuk Alexandr1, Shapoval Oleg M.1, Roddatis Vladimir2, Bruchmann-Bamberg V.3, Samwer Konrad H.3, Moshnyaga Vasily T.3
 
1 Institute of the Electronic Engineering and Nanotechnologies "D. Ghitu" of the Academy of Sciences of Moldova,
2 Institute for Materials Physics, Goettingen,
3 Georg-August-Universitat-Gottingen
 
 
Disponibil în IBN: 18 iulie 2022


Rezumat

We report on the interface engineering in correlated manganite heterostructures by octahedral decoupling using embedded stacks of atomic layers that form the Ruddlesden-Popper structure. A room temperature magnetic decoupling was achieved through deposition of a (SrO)2–TiO2–(SrO)2 sequence of atomic layers at the interface between La0.7Sr0.3MnO3 and La0.7Sr0.3Mn0.9Ru0.1O3 films. Moreover, the narrowing of the interfacial dead layer in ultrathin La0.7Sr0.3MnO3 films was demonstrated by insertion of a single (SrO)2 rock-salt layer at the interface with the SrTiO3(100) substrate. The obtained results are discussed based on the symmetry breaking and disconnection of the MnO6 octahedra network at the interface that may lead to the improved performance of all-oxide magnetic tunnel junctions. We suggest that octahedral decoupling realized by formation of Ruddlesden-Popper interfaces is an effective structural mechanism to control functionalities of correlated perovskite heterostructures.The authors acknowledge financial support by the Deutsche Forschungsgemeinschaft (DFG) via SFB 1073 (TP B04, B01).

Cuvinte-cheie
magnetism, manganese, manganese oxide, manganites, Tunnel junctions, Ultrathin films