Thermoelectric properties of electrically gated bismuth telluride nanowires
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BEJENARI, Igor, KANTSER, Valeriu, BALANDIN, Alexander A.. Thermoelectric properties of electrically gated bismuth telluride nanowires. In: Physical Review B - Condensed Matter and Materials Physics, 2010, vol. 81, p. 0. ISSN 1098-0121. DOI: https://doi.org/10.1103/PhysRevB.81.075316
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Physical Review B - Condensed Matter and Materials Physics
Volumul 81 / 2010 / ISSN 1098-0121 /ISSNe 1550-235X

Thermoelectric properties of electrically gated bismuth telluride nanowires

DOI:https://doi.org/10.1103/PhysRevB.81.075316

Pag. 0-0

Bejenari Igor12, Kantser Valeriu2, Balandin Alexander A.1
 
1 University of California, Riverside,
2 Institute of Electronic Engineering and Industrial Technologies, Academy of Sciences of Moldova
 
 
Disponibil în IBN: 25 iunie 2023


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We theoretically studied how the electric field effect can modify thermoelectric properties of intrinsic, n -type and p -type bismuth telluride nanowires with the growth direction [110]. The electronic structure and the wave functions were calculated by solving self-consistently the system of the Schrödinger and Poisson equations using the spectral method. The Poisson equation was solved in terms of the Newton-Raphson method using the predictor-corrector approach. The electron-electron exchange-correlation interaction was taken into account in our analysis. In the temperature range from 77 to 500 K, the dependences of the Seebeck coefficient, thermal conductivity, electron (hole) concentration, and thermoelectric figure of merit on the nanowire thickness, gate voltage, and excess hole (electron) concentration were investigated in the constant relaxation-time approximation. The results of our calculations indicate that the external perpendicular electric field can increase the Seebeck coefficient of the bismuth telluride nanowires with thicknesses of 7-15 nm by nearly a factor of 2 and enhance ZT by an order of magnitude. At room temperature, ZT can reach a value as high as 3.4 under the action of the external perpendicular electric field for realistic widths of the nanowires. The obtained results may open up a way for a drastic enhancement of the thermoelectric figure of merit in a wide temperature range.