Nonequilibrium dynamics of α-RuCl3 - a time-resolved magneto-optical spectroscopy study
Закрыть
Conţinutul numărului revistei
Articolul precedent
Articolul urmator
242 0
SM ISO690:2012
WAGNER, Julian, SAHASRABUDHE, Anuja, VERSTEEG, Rolf B., WANG, Zhe, TSURKAN, Vladimir, LOIDL, Alois, HEDAYAT, Hamoon, VAN LOOSDRECHT, Paul H.M.M.. Nonequilibrium dynamics of α-RuCl3 - a time-resolved magneto-optical spectroscopy study. In: Faraday Discussions, 2022, nr. 237, pp. 237-258. ISSN 1359-6640. DOI: https://doi.org/10.1039/d2fd00006g
EXPORT metadate:
Google Scholar
Crossref
CERIF

DataCite
Dublin Core
Faraday Discussions
Numărul 237 / 2022 / ISSN 1359-6640 /ISSNe 1364-5498

Nonequilibrium dynamics of α-RuCl3 - a time-resolved magneto-optical spectroscopy study

DOI:https://doi.org/10.1039/d2fd00006g

Pag. 237-258

Wagner Julian1, Sahasrabudhe Anuja1, Versteeg Rolf B.1, Wang Zhe2, Tsurkan Vladimir34, Loidl Alois3, Hedayat Hamoon, Van Loosdrecht Paul H.M.M.1
 
1 University of Cologne,
2 Technical University of Dortmund,
3 University of Augsburg,
4 Institute of Applied Physics
 
 
Disponibil în IBN: 24 noiembrie 2022


Rezumat

We present time-resolved magneto-optical spectroscopy on the magnetic Mott-Hubbard-insulating Kitaev spin liquid candidate α-RuCl3 to investigate the nonequilibrium dynamics of its antiferromagnetically ordered zigzag groundstate after photoexcitation. A systematic study of the transient magnetic linear dichroism under different experimental conditions (temperature, external magnetic field, photoexcitation density) gives direct access to the dynamical interplay of charge excitations with the zigzag ordered state on ultrashort time scales. We observe a rather slow initial demagnetization (few to 10s of ps) followed by a long-lived non-thermal antiferromagnetic spin-disordered state (100-1000s of ps), which can be understood in terms of holons and doublons disordering the antiferromagnetic background after photoexcitation. Varying temperature and fluence in the presence of an external magnetic field reveals two distinct photoinduced dynamics associated with the zigzag and quantum paramagnetic disordered phases. The photo-induced non-thermal spin-disordered state shows universal compressed-exponential recovery dynamics related to the growth and propagation of zigzag domains on nanosecond time scales, which is interpreted within the framework of the Fatuzzo-Labrune model for magnetization reversal. The study of nonequilibrium states in strongly correlated materials is a relatively unexplored topic, but our results are expected to be extendable to a large class of Mott-Hubbard insulator materials with strong spin-orbit coupling.

Cuvinte-cheie
Antiferromagnetism, Dichroism, Dynamics, Magnetic fields, Photoexcitation, Spin dynamics