Experimental evidence for competition between antiferromagnetic and ferromagnetic correlations in HgCr2 S4
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TSURKAN, Vladimir, HEMBERGER, Joachim, KRIMMEL, Alexander, KRUG VON NIDDA, Hans Albrecht, LUNKENHEIMER, Peter, WEBER, S., ZESTREA, Veaceslav, LOIDL, Alois. Experimental evidence for competition between antiferromagnetic and ferromagnetic correlations in HgCr2 S4. In: Physical Review B - Condensed Matter and Materials Physics, 2006, vol. 73, p. 0. ISSN 1098-0121. DOI: https://doi.org/10.1103/PhysRevB.73.224442
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Physical Review B - Condensed Matter and Materials Physics
Volumul 73 / 2006 / ISSN 1098-0121 /ISSNe 1550-235X

Experimental evidence for competition between antiferromagnetic and ferromagnetic correlations in HgCr2 S4

DOI:https://doi.org/10.1103/PhysRevB.73.224442

Pag. 0-0

Tsurkan Vladimir12, Hemberger Joachim1, Krimmel Alexander1, Krug Von Nidda Hans Albrecht1, Lunkenheimer Peter1, Weber S.1, Zestrea Veaceslav2, Loidl Alois1
 
1 Center for Electronic Correlations and Magnetism, University of Augsburg,
2 Institute of Applied Physics, Academy of Sciences of Moldova
 
 
Disponibil în IBN: 27 iunie 2023


Rezumat

A detailed study of polycrystalline and single crystalline samples of the normal spinel HgCr2 S4 is reported. The structural refinement reveals enhanced values of the atomic displacements suggesting the closeness to a structural instability. Magnetization, electron-spin resonance, and specific-heat studies document strong ferromagnetic fluctuations close to 50 K and the occurrence of complex antiferromagnetic order at TN =22 K. We found highly unconventional behavior resembling properties of a noncollinear antiferromagnet and of a soft ferromagnet dependent on temperature and magnetic field. Even weak external magnetic fields disturb the antiferromagnetic order and strongly enhance the ferromagnetic correlations. The observed anomalies are related to bond frustration due to competing magnetic exchange interactions between the Cr ions. 

Cuvinte-cheie
magnetism, Curie Temperature, Antiferromagnet