Magnetic ground state and two-dimensional behavior in pseudo-kagome layered system Cu 3Bi(SeO 3) 2O 2Br
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PREGELJ, Matej, ZAHARKO, Oksana, GUNTHER, A., LOIDL, Alois, TSURKAN, Vladimir, GUERRERO, Sebastian. Magnetic ground state and two-dimensional behavior in pseudo-kagome layered system Cu 3Bi(SeO 3) 2O 2Br. In: Physical Review B - Condensed Matter and Materials Physics, 2012, vol. 86, p. 0. ISSN 1098-0121. DOI: https://doi.org/10.1103/PhysRevB.86.144409
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Physical Review B - Condensed Matter and Materials Physics
Volumul 86 / 2012 / ISSN 1098-0121 /ISSNe 1550-235X

Magnetic ground state and two-dimensional behavior in pseudo-kagome layered system Cu 3Bi(SeO 3) 2O 2Br

DOI:https://doi.org/10.1103/PhysRevB.86.144409

Pag. 0-0

Pregelj Matej12, Zaharko Oksana2, Gunther A.3, Loidl Alois3, Tsurkan Vladimir34, Guerrero Sebastian2
 
1 Jozef Stefan Institute,
2 Paul Scherrer Institute,
3 Center for Electronic Correlations and Magnetism, University of Augsburg,
4 Institute of Applied Physics, Academy of Sciences of Moldova
 
 
Disponibil în IBN: 26 iunie 2023


Rezumat

Anisotropic magnetic properties of a layered kagome-like system Cu 3Bi(SeO 322Br have been studied by bulk magnetization and magnetic susceptibility measurements as well as powder and single-crystal neutron diffraction. At T N=27.4 K the system develops an alternating antiferromagnetic order of (ab) layers, which individually exhibit canted ferrimagnetic moment arrangement, resulting from the competing ferro- and antiferro-magnetic intralayer exchange interactions. A magnetic field B C∼0.8 T applied along the c axis (perpendicular to the layers) triggers a metamagnetic transition, when every second layer flips, i.e., resulting in a ferrimagnetic structure. Significantly higher fields are required to rotate the ferromagnetic component towards the b axis (∼7T) or towards the a axis (∼15T). The estimates of the exchange coupling constants and features indicative of an XY character of this quasi-2D system are presented. 

Cuvinte-cheie
Nonlinear optics, Optical materials, Second harmonic generation