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SM ISO690:2012 BACHUS, Sebastian, KAIB, David A.S., JESCHE, Anton, TSURKAN, Vladimir, LOIDL, Alois, WINTER, Stephen M., TSIRLIN, Alexander A., VALENTI , Roser, GEGENWART, Philipp. Angle-dependent thermodynamics of α-RuCl3. In: Physical Review B, 2021, vol. 103, p. 0. ISSN 2469-9950. DOI: https://doi.org/10.1103/PhysRevB.103.054440 |
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Physical Review B | ||||||
Volumul 103 / 2021 / ISSN 2469-9950 /ISSNe 2469-9969 | ||||||
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DOI:https://doi.org/10.1103/PhysRevB.103.054440 | ||||||
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Thermodynamics of the Kitaev honeycomb magnet α-RuCl3 is studied for different directions of in-plane magnetic field using measurements of the magnetic Grüneisen parameter ΓB and specific heat C. We identify two critical fields BcAF1 and BcAF2 corresponding, respectively, to a transition between two magnetically ordered states and the loss of magnetic order toward a quantum paramagnetic state. The BcAF2 phase boundary reveals a narrow region of magnetic fields where inverse melting of the ordered phase may occur. No additional transitions are detected above BcAF2 for any direction of the in-plane field, although a shoulder anomaly in ΓB is observed systematically at 8-10T. Large field-induced entropy effects imply additional low-energy excitations at low fields and/or strongly field-dependent phonon entropies. Our results establish universal features of α-RuCl3 in high magnetic fields and challenge the presence of a field-induced Kitaev spin liquid in this material. |
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Cuvinte-cheie entropy, Magnetic fields, specific heat |
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