Photoinduced long-lived state in FeSe0.4Te0.6
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FANFARILLO, Laura, KOPIC, Damir, STERZI, Andrea, MANZONI, Giulia, CREPALDI, Alberto, PAYNE, Daniel T., BRONSCH, Wibke, TSURKAN, Vladimir, CROITORI, Dorina, DEISENHOFER, Joachim, PARMIGIANI, Fulvio, CAPONE, Massimo, CILENTO, Federico. Photoinduced long-lived state in FeSe0.4Te0.6. In: Journal of Electron Spectroscopy and Related Phenomena, 2021, nr. 250, p. 0. ISSN 0368-2048. DOI: https://doi.org/10.1016/j.elspec.2021.147090
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Journal of Electron Spectroscopy and Related Phenomena
Numărul 250 / 2021 / ISSN 0368-2048

Photoinduced long-lived state in FeSe0.4Te0.6

DOI:https://doi.org/10.1016/j.elspec.2021.147090

Pag. 0-0

Fanfarillo Laura12, Kopic Damir3, Sterzi Andrea3, Manzoni Giulia3, Crepaldi Alberto4, Payne Daniel T.5, Bronsch Wibke5, Tsurkan Vladimir67, Croitori Dorina7, Deisenhofer Joachim6, Parmigiani Fulvio8, Capone Massimo2, Cilento Federico5
 
1 University of Florida,
2 International School for Advanced Studies (SISSA), Trieste,
3 University of Trieste,
4 Swiss Federal Institute of Technology Lausanne,
5 Elettra Synchrotron Trieste,
6 University of Augsburg,
7 Institute of Applied Physics,
8 University of Cologne
 
 
Disponibil în IBN: 14 iulie 2021


Rezumat

FeSexTe1−x compounds display a rich phase diagram, ranging from the nematicity of FeSe to the (π,π) magnetism of FeTe. We focus on FeSe0.4Te0.6, and exploit tr-ARPES to study its ultrafast electron dynamics following photoexcitation by near-infrared pump pulses. By exploiting probe-polarization-dependent matrix element effects, we reveal a photoinduced long-lived state, lasting for a few tens of picoseconds, showing features compatible with a nematic state. The possibility to induce a long-lived state in this compound by using ultra-short pulses might shed a new light on the driving force behind the nematic symmetry breaking in iron-based superconductors. With the aid of a phenomenological model, we illustrate how our results possibly question the common belief that a low-energy coupling with fluctuations is a necessary condition to stabilize the nematic order. On the contrary, the tendency towards orbital differentiation due to strong electronic correlations induced by the Hund's coupling could be at the origin of the nematic order in iron-based superconductors. 

Cuvinte-cheie
FeSe, FeSeTe, Nematicity, phase transition, TR-ARPES, Ultrafast