Magnetic field dependence of low-energy magnons, anisotropic heat conduction, and spontaneous relaxation of magnetic domains in the cubic helimagnet ZnCr2Se4
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INOSOV, Dmytro S., ONYKIIENKO, Y. A., TYMOSHENKO, Y. V., AKOPYAN, A., SHUKLA, Dharmendra, PRASAI, Narayan, DOERR, Mathias, GORBUNOV, Denis, ZHERLITSYN, S., VONESHEN, David J., BOEHM, Martin, TSURKAN, Vladimir, FELEA, Viorel, LOIDL, Alois, COHN, Joshua L.. Magnetic field dependence of low-energy magnons, anisotropic heat conduction, and spontaneous relaxation of magnetic domains in the cubic helimagnet ZnCr2Se4. In: Physical Review B, 2020, vol. 102, p. 0. ISSN 2469-9950. DOI: https://doi.org/10.1103/PhysRevB.102.184431
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Physical Review B
Volumul 102 / 2020 / ISSN 2469-9950 /ISSNe 2469-9969

Magnetic field dependence of low-energy magnons, anisotropic heat conduction, and spontaneous relaxation of magnetic domains in the cubic helimagnet ZnCr2Se4

DOI:https://doi.org/10.1103/PhysRevB.102.184431

Pag. 0-0

Inosov Dmytro S.1, Onykiienko Y. A.1, Tymoshenko Y. V.1, Akopyan A.2, Shukla Dharmendra2, Prasai Narayan2, Doerr Mathias1, Gorbunov Denis3, Zherlitsyn S.3, Voneshen David J.4, Boehm Martin5, Tsurkan Vladimir67, Felea Viorel7, Loidl Alois6, Cohn Joshua L.2
 
1 Technische Universitat Dresden, Dresden,
2 Miami University,
3 Helmholtz-Zentrum Dresden-Rossendorf,
4 Rutherford Appleton Laboratory, Harwell Oxford,
5 Institut Laue-Langevin, Grenoble,
6 University of Augsburg,
7 Institute of Applied Physics
 
 
Disponibil în IBN: 12 martie 2021


Rezumat

Anisotropic low-temperature properties of the cubic spinel helimagnet ZnCr2Se4 in the single-domain spin-spiral state are investigated by a combination of neutron scattering, thermal conductivity, ultrasound velocity, and dilatometry measurements. In an applied magnetic field, neutron spectroscopy shows a complex and nonmonotonic evolution of the spin-wave spectrum across the quantum-critical point that separates the spin-spiral phase from the field-polarized ferromagnetic phase at high fields. A tiny spin gap of the pseudo-Goldstone magnon mode, observed at wave vectors that are structurally equivalent but orthogonal to the propagation vector of the spin helix, vanishes at this quantum critical point, restoring the cubic symmetry in the magnetic subsystem. The anisotropy imposed by the spin helix has only a minor influence on the lattice structure and sound velocity but has a much stronger effect on the heat conductivities measured parallel and perpendicular to the magnetic propagation vector. The thermal transport is anisotropic at T2K, highly sensitive to an external magnetic field, and likely results directly from magnonic heat conduction. We also report long-time thermal relaxation phenomena, revealed by capacitive dilatometry, which are due to magnetic domain motion related to the destruction of the single-domain magnetic state, initially stabilized in the sample by the application and removal of magnetic field. Our results can be generalized to a broad class of helimagnetic materials in which a discrete lattice symmetry is spontaneously broken by the magnetic order.

Cuvinte-cheie
Anisotropy, Chromium compounds, Crystal lattices, Dilatometers, Heat conduction, Magnetic fields, Neutron scattering, Selenium compounds, Spin waves, temperature, thermal conductivity, Zinc compounds