Magnetic anisotropy and exchange paths for octahedrally and tetrahedrally coordinated Mn2+ ions in the honeycomb multiferroic Mn2Mo3O8
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SZALLER, David, SZASZ, Krisztian, BORDACS, Sandor, VIIROK, Johan, ROOM, Toomas, NAGEL, Urmas, SHUVAEV, Alexey M., WEYMANN, Lukas, PIMENOV, Andrei G., TSIRLIN, Alexander A., JESCHE, Anton, PRODAN, Lilian, TSURKAN, Vladimir, KEZSMARKI, Istvan. Magnetic anisotropy and exchange paths for octahedrally and tetrahedrally coordinated Mn2+ ions in the honeycomb multiferroic Mn2Mo3O8. In: Physical Review B, 2020, vol. 102, p. 0. ISSN 2469-9950. DOI: https://doi.org/10.1103/PhysRevB.102.144410
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Physical Review B
Volumul 102 / 2020 / ISSN 2469-9950 /ISSNe 2469-9969

Magnetic anisotropy and exchange paths for octahedrally and tetrahedrally coordinated Mn2+ ions in the honeycomb multiferroic Mn2Mo3O8

DOI:https://doi.org/10.1103/PhysRevB.102.144410

Pag. 0-0

Szaller David1, Szasz Krisztian2, Bordacs Sandor23, Viirok Johan4, Room Toomas4, Nagel Urmas4, Shuvaev Alexey M.1, Weymann Lukas1, Pimenov Andrei G.1, Tsirlin Alexander A.5, Jesche Anton5, Prodan Lilian65, Tsurkan Vladimir65, Kezsmarki Istvan5
 
1 Vienna University of Technology,
2 Budapest University of Technology and Economics, Department of Physics, Budapest,
3 Hungarian Academy of Sciences,
4 National Institute of Chemical Physics and Biophysics, Tallinn,
5 University of Augsburg,
6 Institute of Applied Physics
 
 
Disponibil în IBN: 6 noiembrie 2020


Rezumat

We investigated the static and dynamic magnetic properties of the polar ferrimagnet Mn2Mo3O8 in three magnetically ordered phases via magnetization, magnetic torque, and THz absorption spectroscopy measurements. The observed magnetic field dependence of the spin-wave resonances, including Brillouin zone-center and zone-boundary excitations, magnetization, and torque, are well described by an extended two-sublattice antiferromagnetic classical mean-field model. In this orbitally quenched system, the competing weak easy-plane and easy-axis single-ion anisotropies of the two crystallographic sites are determined from the model and assigned to the tetrahedral and octahedral sites, respectively, by ab initio calculations. 

Cuvinte-cheie
Absorption spectroscopy, Calculations, crystallography, magnetization, Manganese compounds, Mean field theory, Molybdenum compounds, multiferroics, multilayers, Spin waves, Terahertz spectroscopy